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Beilstein J. Org. Chem. 2019, 15, 1107–1115, doi:10.3762/bjoc.15.107
Graphical Abstract
Scheme 1: Previously developed bis-nucleophile/bis-electrophile [3 + 2] annulations.
Scheme 2: Concept: [3 + 2] C–C/C–C vs C–C/O–C bond-forming annulations.
Figure 1: Examples of annulated cylopentanic (top) and furan-based (bottom) substructures in natural products....
Scheme 3: C–C/O–C bond forming annulations with dimethyl 3-oxoglutarate (1a).
Scheme 4: C–C/C–C bond-forming annulations with dimethyl 3-oxoglutarate (1a).
Scheme 5: C–C/C–O bond-forming annulations with various bis-nucleophiles.
Scheme 6: Decarboxylative rearrangement of 4a into 5a.
Scheme 7: Proposed mechanism for the Pd-catalyzed part of the [3 + 2] annulation reaction.
Scheme 8: Proposed mechanism for the temperature dependent cyclization part of the [3 + 2] annulation.
Beilstein J. Org. Chem. 2018, 14, 3059–3069, doi:10.3762/bjoc.14.284
Figure 1: Structures and MICs of Pt-based compounds against P. aeruginosa PAO1.
Figure 2: Transcriptomic analysis of control and cisplatin-treated PAO1 cultures. Heatmap comparing the trans...
Figure 3: Function enrichment of differentially expressed genes from the transcriptomic analysis. A dot-lot f...
Figure 4: Cisplatin fast-kill assay against the P. aeruginosa PAO1, ΔrecA mutant and the ΔrecACOM strain. P. ...
Figure 5: Cisplatin treatment represses T3SS associated virulence. (A) Cisplatin treatment downregulated the ...
Figure 6: P. aeruginosa biofilm killing assay by cisplatin, tobramycin and their combinations. P. aeruginosa ...
Figure 7: Cisplatin treatment attenuates P. aeruginosa infections. CFU mL−1 of PAO1 obtained from corneas wit...